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After working with modern architect Walter Gropius at the Architects ' Collaborative, Gund began his career with significant projects that drew from a modernist vocabulary.

The Hyatt Regency Cambridge, with its stepped massing, recalled legendary projects by architects Adolf Loos and Henri Sauvage, while utilizing red brick characteristic of Cambridge's collegiate river-side architecture.

For Boston's Institute for Contemporary Art, Gund created an unexpected, open, angular interior that played against the rigid geometry of a historic Richardsonian Romanesque building.