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James Harrison of the Pittsburgh Steelers set the record for the longest interception return for a touchdown in a Super Bowl in Super Bowl XLIII.
Coincidently, it is also the Super Bowl's longest play in history ( no other play, such as a fumble return or kick return has been 100 yards ).
The NFL's Defensive Player of the Year Harrison picked off Kurt Warner's pass and returned it a Super Bowl-record 100 yards for a touchdown on the final play of the first half to give the Pittsburgh Steelers a 17-7 lead over the Arizona Cardinals.

2.083 seconds.