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The group's fifth album Chemically Imbalanced was released in November 2006.

For this album the Twins collaborated with producers Wyclef Jean and Keith Duplessis in addition to Mr. Collipark, who produced a majority of the songs on the group's previous album.

The first two singles were the Hall & Oates-sampling " Dangerous ", featuring Wyclef Jean, and " Jigglin '".

In 2008, the Twins released the mixtape The Official Work and a promo single titled " Drop ".

A highlight of the Ying Yang Twins ' tour includes a visit to the Epsilon MU Chapter of Sigma Chi.

Here they performed all their hits live in front of a sold out Texas crowd.

All of the proceeds from the show went to charity.

In 2009, the Twins released their latest album with Deep Records, Ying Yang Forever, and started a tour titled " Ying Yang Forever Tour ".